Actors who have portrayed Satan

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  • Al Pacino in The Devil's Advocate
  • Harvey Keitel in Little Nickey
  • Elizabeth Hurley in Bedazzled
  • Rosalinda Celentano in the Passion of the Christ
  • Trey Parker (Voice) on South Park
  • Jim Fortier (Voice) on Aqua Teen Hungar Force
  • Jose Luis Aguirre in Santa Claus
  • Robert de Niro in Angel Heart
  • Jack Nicholson in The Witches of Eastwick
  • Victor Buono in The Evil (1981).
  • Peter Cook in the original Bedazzled
  • Viggo Mortensen in The Prophecy ('95).
Author Comments: 

..or the Devil...yadda yadda. I know I'm missing alot probably, help me out if you please. Thanks, just thought it'd be interesting.

Jose Luis Aguirre as the Devil in Santa Claus

There's also Robert de Niro in "Angel Heart" and Jack Nicholson in "The Witches of Eastwick".

Victor Buono in The Evil (1981).

Also, Mercedes McCambridge did the voice of the demon that possesses Linda Blair in The Exorcist, but that's up to you if it counts.

Oops, forgot an obvious one: Peter Cook in the original Bedazzled (1967).

Viggo Mortensen in The Prophecy ('95). Trying to out-do Christopher Walken doing a Christopher Walken.

George Burns played God and Satan in Oh, God! You Devil (1984).

Bill Cosby in The Devil and Max Devlin

Robin Hughes in episode 41, season 2 of the original Twilight Zone. Episode title: The Howling Man.

Who is Robin Hughes?

Alan Cumming (voice) in the shortlived animated TV series "God, the Devil, and Bob"